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Interconnection of organic–inorganic hybrid nano-building blocks towards thermally robust mesoporous structures

https://hiroshima.repo.nii.ac.jp/records/2007755
https://hiroshima.repo.nii.ac.jp/records/2007755
e3ebb1b4-8674-4c31-85e5-b8279f932e48
名前 / ファイル ライセンス アクション
Nanoscale_13_11446.pdf Nanoscale_13_11446.pdf (4.0 MB)
Item type デフォルトアイテムタイプ_(フル)(1)
公開日 2023-03-18
タイトル
タイトル Interconnection of organic–inorganic hybrid nano-building blocks towards thermally robust mesoporous structures
言語 en
作成者 Tarutani, Naoki

× Tarutani, Naoki

en Tarutani, Naoki

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Sato, Riona

× Sato, Riona

en Sato, Riona

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Yamazaki, Wataru

× Yamazaki, Wataru

en Yamazaki, Wataru

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Katagiri, Kiyofumi

× Katagiri, Kiyofumi

en Katagiri, Kiyofumi

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Inumaru, Kei

× Inumaru, Kei

en Inumaru, Kei

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Ishigaki, Takamasa

× Ishigaki, Takamasa

en Ishigaki, Takamasa

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アクセス権
アクセス権 open access
アクセス権URI http://purl.org/coar/access_right/c_abf2
権利情報
権利情報 This journal is © The Royal Society of Chemistry 2021
権利情報
権利情報 Open Access Article. This article is licensed under a Creative Commons Attribution-NonCommercial 3.0 Unported Licence.
内容記述
内容記述 The use of organic–inorganic hybrid nanoparticles will enable a control of the characteristics of both the nanoparticles and constructed fine structures. In this study, we report the synthesis of acrylate-intercalated layered manganese, cobalt, and nickel hydroxide nanoparticles and their assembly into ordered mesoporous structures. Polymerization of the intercalated acrylates takes place by means of a radical initiator. The formed organic network improved the thermal stability of the layered hydroxides, which results in thermally robust mesoporous structures. Additionally, it is found that the polymerization can be initiated and progressed at 200 °C without any initiators for the layered nickel hydroxide system. This allows for the scalable solid-state thermal polymerization of intercalated acrylates and the formation of thermally robust hierarchically ordered meso/macroporous powders as well as mesoporous films. The electrochemical characterization reveals that the thermally robust mesoporous films having regulated mesopores allow for the effective diffusion of molecules/solvent compared with the films having collapsed mesoporous structures.
言語 en
内容記述
内容記述タイプ Other
内容記述 The present work is partially supported by JSPS KAKENHI Grant Number JP20K15368, JSPS Core-to-Core Program, MEXT Leading Initiative for Excellent Young Researchers, the Foundation for the Promotion of Ion Engineering, International Network on Polyoxometalate Science at Hiroshima University, and the Izumi Science and Technology Foundation (2019-J-112).
出版者
出版者 The Royal Society of Chemistry
言語
言語 eng
資源タイプ
資源タイプ識別子 http://purl.org/coar/resource_type/c_6501
資源タイプ journal article
出版タイプ
出版タイプ VoR
出版タイプResource http://purl.org/coar/version/c_970fb48d4fbd8a85
関連情報
識別子タイプ DOI
関連識別子 10.1039/d0nr08689d
関連情報
識別子タイプ DOI
関連識別子 https://doi.org/10.1039/d0nr08689d
収録物識別子
収録物識別子タイプ ISSN
収録物識別子 2040-3372
開始ページ
開始ページ 11446
書誌情報 Nanoscale
Nanoscale

巻 13, p. 11446-11454, 発行日 2021-06-23
旧ID 52858
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