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Neutron scattering and thermal studies of the Ni-incorporated CeSbNix system

https://hiroshima.repo.nii.ac.jp/records/2008187
https://hiroshima.repo.nii.ac.jp/records/2008187
d229eba4-24c1-42d0-ba4f-44271599eb5c
名前 / ファイル ライセンス アクション
PhysRevB_62_12181.pdf PhysRevB_62_12181.pdf (158.1 KB)
Item type デフォルトアイテムタイプ_(フル)(1)
公開日 2023-03-18
タイトル
タイトル Neutron scattering and thermal studies of the Ni-incorporated CeSbNix system
言語 en
作成者 Adroja, D. T.

× Adroja, D. T.

en Adroja, D. T.

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Armitage, J. G. M.

× Armitage, J. G. M.

en Armitage, J. G. M.

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Riedi, P. C.

× Riedi, P. C.

en Riedi, P. C.

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Jung, M. H.

× Jung, M. H.

en Jung, M. H.

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Tun, Z.

× Tun, Z.

en Tun, Z.

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Takabatake, Toshiro

× Takabatake, Toshiro

en Takabatake, Toshiro

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アクセス権
アクセス権 open access
アクセス権URI http://purl.org/coar/access_right/c_abf2
権利情報
権利情報 Copyright (c) 2000 The American Physical Society.
内容記述
内容記述 Neutron scattering, thermal expansion, and magnetostriction measurements have been carried out on the cubic compounds CeSbNix (x=0-0.4). Inelastic neutron scattering studies show a well-defined crystal field (CF) excitation at 4.06 (±0.04) meV and 5.02(±0.05) meV in x=0.08 and 0.15, respectively. The crystal field splitting increases with x compared with the parent compound CeSb (3.19 meV) in spite of the lattice parameter increasing with Ni incorporation. The implication is that the increase in the CF splitting in x=0.08 and 0.15 is due to a collapse of the p-f mixing between the Sb 5p holes and the localized Ce 4f electrons. The analysis of inelastic spectra of x=0.15 shows that the ground state is a doublet (Γ7), which explains the temperature-dependent behavior of the magnetic susceptibility. Thermal expansion shows a dramatic change in behavior with Ni composition. The thermal expansion coefficient exhibits a first-order transition at 15.4 K in CeSb, which disappears for Ni composition as low as x=0.035, as well as in an applied field of 8 T. A large magnetostriction has been observed in CeSb in the magnetic-ordered state as well as in the paramagnetic state. The absolute values of the magnetostriction are reduced considerably in the Ni-incorporated alloys. The volume magnetostriction of x= 0.15 alloy exhibits a scaling behavior in the paramagnetic state from which we have estimated the product of the magnetovolume coupling constant and the isothermal compressibility.
言語 en
出版者
出版者 American Physical Society
言語
言語 eng
資源タイプ
資源タイプ識別子 http://purl.org/coar/resource_type/c_6501
資源タイプ journal article
出版タイプ
出版タイプ VoR
出版タイプResource http://purl.org/coar/version/c_970fb48d4fbd8a85
関連情報
識別子タイプ DOI
関連識別子 10.1103/PhysRevB.62.12181
関連情報
識別子タイプ DOI
関連識別子 http://dx.doi.org/10.1103/PhysRevB.65.014406
収録物識別子
収録物識別子タイプ ISSN
収録物識別子 1098-0121
収録物識別子
収録物識別子タイプ NCID
収録物識別子 AA11187113
開始ページ
開始ページ 12 181
書誌情報 Physical Review B - Condensed Matter and Materials Physics
Physical Review B - Condensed Matter and Materials Physics

巻 62, 号 18, p. 12 181-12 189, 発行日 2000-11-01
旧ID 19304
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